i love gilear and plug as much as anyone else but here are some of my favorite npcs that imo people don't talk about enough. maybe part 2 in the future

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Junkmother (A Starstruck Odyssey)
Garbanzo Buglass (Tiny Heist)
Justin Fication (Mentopolis)
Nona (The Seven)
Percival/Stalker (Escape From the Bloodkeep)